Mathematical Modeling and Analysis
We have demonstrated, in a periodically forced oscillatory Belousov-Zhabotinsky reaction and in mathematical models, a mechanism for creating spatio-temporal disorder. The mechanism consists of the creation of spiral vortex pairs through a transverse instability of fronts in the vicinity of a nonequilibrium Ising-Bloch bifurcation. We used an amplitude equation model, the forced complex Ginzburg-Landau equation, to reproduce the experimental observations with numerical solutions, and further described the mechanism for vortex creation with the normal form equations for a curved front line.